温度对煤层气井用低密陶粒支撑剂性能的影响Effects of Temperature on Properties of Low-density Ceramic Proppants Used in Coalbed Methane Wells
雷宏娇,田玉明,宋伟,唐睿,白频波
摘要(Abstract):
以铝矾土和煤矸石为主要原料,加以钾长石为助烧结剂,在不同温度下烧结制备30/50目煤层气井用陶粒支撑剂。使用X射线衍射(XRD)和扫描电子显微镜(SEM)对陶粒支撑剂样品进行物相组成和微观形貌表征,同时研究了烧结温度对陶粒微观结构与力学性能的影响。结果表明:陶粒内部形成了大量闭气孔,导致陶粒随烧结温度的升高,其密度和抗压能力呈下降趋势。1 260℃下烧结制备的陶粒支撑剂综合性能较好,其视密度为2.34 g/cm~3,体积密度1.20 g/cm~3,28 MPa闭合压力下的破碎率5.12%,即满足破碎率要求的同时保持低密,在该温度下烧结制备的陶粒支撑剂,棒状莫来石晶相发育良好,数量较多,形成连续的网状结构。
关键词(KeyWords): 煤矸石;煤层气;低密;低温;陶粒支撑剂
基金项目(Foundation): 山西省科技重大专项(20181101001)
作者(Author): 雷宏娇,田玉明,宋伟,唐睿,白频波
参考文献(References):
- [1] 孙杰,王佟,赵欣,等.我国煤层气地质特征与研究方向思考[J].中国煤炭地质,2018,30(6):30-34.
- [2] 国家能源局.煤层气开发利用“十三五”规划[J].能源与环境,2017(1):109.
- [3] 李军鹏,刘斌辉,袁雄.浅析煤层气增产措施[J].内蒙古煤炭经济,2019(21):171-172.
- [4] WU T T,ZHOU J,WU B L.Effect of TiO2 content on the acid resistance of a ceramic proppant[J].Corrosion Science,2015,98:716-724.
- [5] QUEIPO N V,VERDE A J,CANELON J,et al.Efficient global optimization for hydraulic fracturing treatment design[J].Journal of Petroleum Science and Engineering,2002,35(3):151-166.
- [6] HAMMOND P S.Settling and slumping in a Newtonian slurry,and implications for proppant placement during hydraulic fracturing of gas wells[J].Chemical Engineering Science,1995,50(20):3247-3260.
- [7] SNEGIREV A I,SLOBODIN B V.Manufacturing process and properties of spherical granules in the MgO-Al2O3-SiO2 system[J].Refractories and Industrial Ceramics,1998,39(9-10):372-374.
- [8] REINICKE A,RYBACKI E,STANCHITS S,et al.Hydraulic fracturing stimulation techniques and formation damage mechanisms-implications from laboratory testing of tight sandstone-proppant systems[J].Geochemistry,2010,70:107-117.
- [9] 力国民,常鑫,朱保顺,等.烧结温度对添加复合助剂制备莫来石-刚玉基陶粒支撑剂性能的影响[J].人工晶体学报,2018,47(9):1850-1854.
- [10] HAO J Y,MA H Q,FENG X,at el.Microstructure and fracture mechanism of low density ceramic proppants[J].Materials Letters,2018,213:92-94.
- [11] 时伟,桑树勋,周效志,等.沁水盆地南部高阶煤储层垂直压裂缝导流能力分析[J].煤田地质与勘探,2011,39(3):19-23+28.
- [12] 郭建春,卢聪,赵金洲,等.支撑剂嵌入程度的实验研究[J].煤炭学报,2008,33(6):661-664.
- [13] 宋绍雷,甄强,王方方,等.低品位煤矸石制备多孔莫来石研究[J].耐火材料,2014,48(1):18-21.
- [14] YI C,MA H Q,CHEN H Y,et al.Preparation and characterization of coal gangue geopolymers[J].Construction and Building Materials,2018,187:318-326.
- [15] 牟军,薛屺,董朋朋,等.铝矾土空心陶粒支撑剂的制备及性能研究[J].人工晶体学报,2017,46(7):1244-1249.
- [16] 秦梅,郝惠兰,田玉明,等.基于煤层气井用陶粒支撑剂的制备[J].硅酸盐通报,2019,38(10):3355-3359.
- [17] 郝海金,陈召英,鲁博.我国煤层气(煤矿瓦斯)抽采利用现状及对其发展的思考[J].山西煤炭,2019,39(4):1-9+23.
- [18] 国家能源局.SY/T 5108-2014水力压裂和砾石充填作业用支撑剂性能测试方法[S].2015.
- [19] 朱文.浅谈印度钾长石的特性及其工业应用[J].佛山陶瓷,2016,26(2):32-36.
- [20] TIAN X R,WU B L,LI J.The exploration of making acidproof fracturing proppants using red mud[J].Journal of Hazardous Materials,2008,160(2):589-593.
- [21] 王晋槐,张玉军.煤矸石对焦宝石基低密度高强度陶粒支撑剂性能的影响[J].现代技术陶瓷,2016,37(2):138-144.
- [22] 高云峰,黄彪,田玉明,等.长石添加量对陶粒支撑剂性能的影响[J].太原科技大学学报,2020,41(5):369-372.
- [23] 武雅乔,王凯悦,田玉明,等.白云石对焦宝石陶粒晶粒发育及性能的影响[J].硅酸盐通报,2017,36(5):1524-1529.